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You can recruit Cait by clearing the location called Combat Zone and talking to her. She is an ex-raider will have a contrasting attitude towards moral decisions. She is also a potential romance partner after maxing out her affinity.
Extra skill/ability
Prior to completing her companion quest, she can actively use chems in her inventory, further boosting her Combat capability.
Cait can be ordered to pick the locks of any difficulty. However, she'll need bobby pins in her inventory to do it. The success and time needed to pick the lock will depend on difficulty. Master locks are particularly challenging, even to her. You can always quicksave before ordering her to attempt picking a lock so you can always reload your game if the attempt fails.