What balls would be usefull to capture Entei, raikou, and Suicune except the ultra ball and the master ball.
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Only other ones I can think of are a Quick Ball, but you'll have to use that on the first try. If you can get them to stick around with Mean Look, a Timer Ball, but that only gets really effective after 40 turns.
If you have you're first Pokemon whos level is higher than raikou entei and suicune by at least 10 levels you could use level balls. If you give kurt red apricorns and come back the next day he will give you level a ball/s
The Ultra ball is the best. Use a Pokemon that can put them to sleep, and you'll have a much easier time.
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