I tryed to get them but it didn't work
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Hmmm lets see....If I understand correctly your meaning that when your going up against the trainers that have them, simple you lower their Hp enough so that you can catch them...put them to sleep or paralyze them then use Ultra Balls...you don't get the master ball until later but then personally I wouldnt use it until you come up against a pokemn impossible to catch. Oh and another thing don't save after you kill one save before it and start over. Hope this helped.
Do oyu know where they are, if not here are the locations. Entei is at the Mt.Battle when it's in trouble, Suicune is in the under when you verse Venus and Raikou is at the shadow pokemon lab. You catch them by putting them to sleep and slowly taking the hp down. Use ultraballs and save after you catch each one.
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