The Best Way To Catch Any Legendary Pokemon
1. Lower the Legendary Pokemon's HP "into the red". This makes catching it easier.
2. Make the Legendary Pokemon Fall Asleep. This too will make it easier to catch.
3. Throw Ultra Balls at the Legendary Pokemon.
4. If it should wake up, make it fall back asleep and continue to throw Ultra Balls. Repeat this process anytime the Legendary Pokemon should wake up.
More tricks, tips and cheats for this game are right here - Pokemon Silver cheats
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