After You Got The Sapphie And Emerald, What Else Is There To Do, I'm Not Sure How To Let The Legendary Dogs Free...
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First of all you get the Sapphire and the Ruby. The dogs are set free depending on which Pokemon you started with. (Beat the Elite 4 twice and then if you started with Squirtle you can catch Raikou, Charmander-Suicune and Bulbasaur-Entei.)
They will apear randomly in Grass or water but not on the Sevii Islands.
I found Raikou when I had beaten all trainers and went for a swim, it will go black for a second longer than normal and it will appear.
Be careful! They run away easily, so use either a Wobbuffet with Shadow Tag as it's power or a Diglett/Dugtrio with Arena Trap, that will stop them from fleeing.
Good luck!
After you unlock the national dex the dogs are freed automaticaly
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